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Precision measurement of 65Zn electron-capture decays with the KDK coincidence setup
Nuclear Data Sheets ( IF 3.7 ) Pub Date : 2023-05-08 , DOI: 10.1016/j.nds.2023.04.003
L. Hariasz , P.C.F. Di Stefano , M. Stukel , B.C. Rasco , K.P. Rykaczewski , N.T. Brewer , R.K. Grzywacz , E.D. Lukosi , D.W. Stracener , M. Mancuso , F. Petricca , J. Ninkovic , P. Lechner

65Zn is a common calibration source, moreover used as a radioactive tracer in medical and biological studies. In many cases, γ-spectroscopy is a preferred method of 65Zn standardization, which relies directly on the branching ratio of Jπ(65Zn) = 5/2 → Jπ(65Cu) = 5/2 via electron capture (EC*). We measure the relative intensity of this branch to that proceeding directly to the ground state (EC0) using a novel coincidence technique, finding IEC0/IEC* = 0.9684 ± 0.0018. Re-evaluating the decay scheme of 65Zn by adopting the commonly evaluated branching ratio of Iβ+ = 1.4271(7)% we obtain IEC* = (50.08 ± 0.06)%, and IEC0 = (48.50 ± 0.06)%. The associated 1115 keV gamma intensity agrees with the previously reported NNDC value, and is now accessible with a factor of ∼2 increase in precision. Our re-evaluation removes reliance on the deduction of this gamma intensity from numerous measurements, some of which disagree and depend directly on total activity determination. The KDK experimental technique provides a new avenue for verification or updates to the decay scheme of 65Zn, and is applicable to other isotopes.



中文翻译:

使用 KDK 符合设置精确测量 65Zn 电子捕获衰减

65 Zn 是一种常见的校准源,此外还用作医学和生物学研究中的放射性示踪剂。在许多情况下,γ能谱是65 Zn 标准化的首选方法,它直接依赖于 J π ( 65 Zn) = 5/2 → J π ( 65 Cu) = 5/2 通过电子捕获的分支比(欧共体*)。我们使用一种新颖的巧合技术测量该分支与直接进入基态 (EC 0 ) 的分支的相对强度,发现 I EC 0/IEC* = 0.9684 ± 0.0018。重新评估65的衰减方案Zn 采用通常评估的支化比I β + = 1.4271(7)%,我们得到 IEC* = (50.08 ± 0.06)%,I EC 0 = (48.50 ± 0.06)%。相关的 1115 keV 伽马强度与之前报告的 NNDC 值一致,现在精度提高了约 2 倍。我们的重新评估消除了对从众多测量中推导出这种伽马强度的依赖,其中一些不同意并直接取决于总活动的确定。KDK实验技术为65 Zn衰变方案的验证或更新提供了新途径,并适用于其他同位素。

更新日期:2023-05-08
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