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Porous Nanographenes, Graphene Nanoribbons, and Nanoporous Graphene Selectively Synthesized from the Same Molecular Precursor J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Mamun Sarker, Christoph Dobner, Percy Zahl, Christian Fiankor, Jian Zhang, Anshul Saxena, Narayana Aluru, Axel Enders, Alexander Sinitskii
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Charge Transfer Mechanism on a Cobalt-Polyoxometalate-TiO2 Photoanode for Water Oxidation in Acid J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Fengyi Zhao, Ting Cheng, Xinlin Lu, Nandan Ghorai, Yiwei Yang, Yurii V. Geletii, Djamaladdin G. Musaev, Craig L. Hill, Tianquan Lian
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Droplet Polymer Bilayers for Bioelectronic Membrane Interfacing J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Emily A. Schafer, Joshua J. Maraj, Camryn Kenney, Stephen A. Sarles, Jonathan Rivnay
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Breaking of Lateral Symmetry in Two-Dimensional Crystallization-Driven Self-Assembly on a Surface J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Geyu Lin, Jiawei Tao, Yan Sun, Yan Cui, Ian Manners, Huibin Qiu
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Carbon Nanotubes as a Solid-State Electron Mediator for Visible-Light-Driven Z-Scheme Overall Water Splitting J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Lihua Lin, Yiwen Ma, Nobuyuki Zettsu, Junie Jhon M. Vequizo, Chen Gu, Akira Yamakata, Takashi Hisatomi, Tsuyoshi Takata, Kazunari Domen
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Enzymatic Reaction-Coupled, Cooperative Supramolecular Polymerization J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Angshuman Das, Saikat Ghosh, Ananya Mishra, Arka Som, Vijay Basavaraj Banakar, Sarit S. Agasti, Subi J. George
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Self-Limiting Phase Transition Enabling Reversible Overstoichiometric Li Storage in Ni-Rich Cathodes J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-15 Xin-Hai Meng, Dongdong Xiao, Zi-Yi Zhou, Wen-Zhe Liu, Ji-Lei Shi, Li-Jun Wan, Yu-Guo Guo
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Self-Trapped Exciton Emission in Highly Polar 0D Hybrid Ammonium/Hydronium-Based Perovskites Triggered by Antimony Doping J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Bo Zhou, Feier Fang, Zexiang Liu, Haizhe Zhong, Kang Zhou, Hanlin Hu, Jiacheng Min, Fangyuan Zheng, Shaofan Fang, Jingheng Nie, Jing-Kai Huang, Lain-Jong Li, Henan Li, Yi Wan, Yumeng Shi
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Direct Observation of Gas-Phase Hydroxymethylene: Photoionization and Kinetics Resulting from Methanol Photodissociation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Emily K. Hockey, Nathan McLane, Carles Martí, LeAnh Duckett, David L. Osborn, Leah G. Dodson
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Effect of Dynamic and Preferential Decoration of Pt Catalyst Surfaces by WOx on Hydrodeoxygenation Reactions J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Justin Marlowe, Siddharth Deshpande, Dionisios G. Vlachos, Mahdi M. Abu-Omar, Phillip Christopher
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Oxygen Isotopologues Resolved from Water Oxidation Electrocatalysis by Electron Paramagnetic Resonance Spectroscopy J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Trisha T. Nguyen, Richard I. Sayler, Aaron H. Shoemaker, Jibo Zhang, Stefan Stoll, Jay R. Winkler, R. David Britt, Bryan M. Hunter
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An Unexpected Decrease in Vibrational Entropy of Multicomponent Rutile Oxides J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Yaowen Wang, Xinbo Li, Jipeng Luo, Brian F. Woodfield, Xiyang Wang, Tao Feng, Nan Yin, Quan Shi, Guangshe Li, Liping Li
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Hydrogen on Colloidal Gold Nanoparticles J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Noreen E. Gentry, Aiko Kurimoto, Kai Cui, Jamie L. Cleron, Claire M. Xiang, Sharon Hammes-Schiffer, James M. Mayer
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Palladium-Catalyzed anti-Michael-Type (Hetero)arylation of Acrylamides J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Hirotsugu Suzuki, Ryota Moro, Takanori Matsuda
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Easy Access to Functionalized Indolines and Tetrahydroquinolines via a Photochemical Cascade Cyclization Reaction J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Julian J. Melder, Maxi L. Heldner, Robin Kugler, Levi A. Ziegenhagen, Frank Rominger, Matthias Rudolph, A. Stephen K. Hashmi
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Spinel Nanostructures for the Hydrogenation of CO2 to Methanol and Hydrocarbon Chemicals J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Mengheng Wang, Lanling Zheng, Genyuan Wang, Jiale Cui, Gui-Ling Guan, Yu-Ting Miao, Jian-Feng Wu, Pan Gao, Fan Yang, Yunjian Ling, Xiangxue Luo, Qinghong Zhang, Gang Fu, Kang Cheng, Ye Wang
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Molecular Pseudorotation in Phthalocyanines as a Tool for Magnetic Field Control at the Nanoscale J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Raphael Wilhelmer, Matthias Diez, Johannes K. Krondorfer, Andreas W. Hauser
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Discovery and Characterization of Pyridoxal 5′-Phosphate-Dependent Cycloleucine Synthases J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Abner N. D. Abad, Kaushik Seshadri, Masao Ohashi, David A. Delgadillo, Lygia S. de Moraes, Kyle K. Nagasawa, Mengting Liu, Samuel Johnson, Hosea M. Nelson, Yi Tang
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Enantioselective Access to β-Amino Carbonyls via Ni-Catalyzed Formal Olefin Hydroamidation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Xiang Lyu, Hoimin Jung, Dongwook Kim, Sukbok Chang
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Organ- and Cell-Selective Delivery of mRNA In Vivo Using Guanidinylated Serinol Charge-Altering Releasable Transporters J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Zhijian Li, Laura Amaya, Aloysius Ee, Sean K. Wang, Alok Ranjan, Robert M. Waymouth, Howard Y. Chang, Paul A. Wender
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Copper–Nitroxyl-Catalyzed α-Oxygenation of Cyclic Secondary Amines Including Application to Late-Stage Functionalization J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Christopher M. Hanneman, Jack Twilton, Melissa N. Hall, Nicole C. Goodwin, Jennifer M. Elward, Tessa Lynch-Colameta, Shannon S. Stahl
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Efficient Capture and Electroreduction of Dilute CO2 into Highly Pure and Concentrated Formic Acid Aqueous Solution J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-14 Zhen-Hua Zhao, Jia-Run Huang, Da-Shuai Huang, Hao-Lin Zhu, Pei-Qin Liao, Xiao-Ming Chen
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Isomeric Porous Cu(I) Triazolate Frameworks Showing Periodic and Aperiodic Flexibility for Efficient CO Separation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Chao Wang, Xue-Wen Zhang, Xiao-Xian Chen, Wei-Xiong Zhang, Jie-Peng Zhang
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Colossal Ferroelectric Photovoltaic Effect in Inequivalent Double-Perovskite Bi2FeMnO6 Thin Films J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Xudong Liu, Jie Tu, Yue-Wen Fang, Guoqiang Xi, Hangren Li, Rong Wu, Xiuqiao Liu, Dongfei Lu, Jiushe He, Junwei Zhang, Jianjun Tian, Linxing Zhang
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Stereodivergent Synthesis of 1,4-Dicarbonyl Compounds through Sulfonium Rearrangement: Mechanistic Investigation, Stereocontrolled Access to γ-Lactones and γ-Lactams, and Total Synthesis of Paraconic Acids J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Nicolas G.-Simonian, Philipp Spieß, Margaux Riomet, Boris Maryasin, Immo Klose, Alexander Beaton Garcia, Laurin Pollesböck, Dainis Kaldre, Uroš Todorovic, Julia Minghua Liu, Daniel Kaiser, Leticia González, Nuno Maulide
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Open Cross-gap Gold Nanocubes with Strong, Large-Area, Symmetric Electromagnetic Field Enhancement for On-Particle Molecular-Fingerprint Raman Bioassays J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Jiyeon Kim, Jae-Myoung Kim, Kyungin Choi, Jeong-Eun Park, Jwa-Min Nam
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Unveiling the Multielectron Acceptor Properties of π-Expanded Pyracylene: Reversible Boat to Chair Conversion J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Yikun Zhu, Jan Borstelmann, Oliver Bertleff, John Bergner, Zheng Wei, Christian Neiss, Andreas Görling, Milan Kivala, Marina A. Petrukhina
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Multistate Dynamics and Kinetics of CO2 Activation by Ta+ in the Gas Phase: Insights into Single-Atom Catalysis J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Yang Liu, Milan Ončák, Jennifer Meyer, Shaun G. Ard, Nicholas S. Shuman, Albert A. Viggiano, Hua Guo
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From Quaternary Carbon to Tertiary C(sp3)–Si and C(sp3)–Ge Bonds: Decyanative Coupling of Malononitriles with Chlorosilanes and Chlorogermanes Enabled by Ni/Ti Dual Catalysis J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Zi-Hao Chen, Yu-Qing Zheng, Hong-Gui Huang, Ke-Hao Wang, Jun-Lin Gong, Wen-Bo Liu
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Synergistic Photoenzymatic Catalysis Enables Synthesis of a-Tertiary Amino Acids Using Threonine Aldolases J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Yao Ouyang, Claire G. Page, Catherine Bilodeau, Todd K. Hyster
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Mechanism of Z-Selective Allylic Functionalization via Thianthrenium Salts J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Karina Targos, Achyut R. Gogoi, Ángel Rentería-Gómez, Min Ji Kim, Osvaldo Gutierrez, Zachary K. Wickens
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Palladium-Catalyzed Ligand-Controlled Switchable Hetero-(5 + 3)/Enantioselective [2σ+2σ] Cycloadditions of Bicyclobutanes with Vinyl Oxiranes J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Jin-Lan Zhou, Yuanjiu Xiao, Linke He, Xin-Yu Gao, Xue-Chun Yang, Wen-Biao Wu, Guoqiang Wang, Junliang Zhang, Jian-Jun Feng
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Multicomponent, Multicavity Metallacages That Contain Different Binding Sites for Allosteric Recognition J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Haifei Liu, Chenxing Guo, Luqi Li, Zeyuan Zhang, Yali Hou, Chaoqun Mu, Gao-lei Hou, Zhenyi Zhang, Heng Wang, Xiaopeng Li, Mingming Zhang
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Mechanism of Electrocatalytic H2 Evolution, Carbonyl Hydrogenation, and Carbon–Carbon Coupling on Cu J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Hongwen Chen, Jayendran Iyer, Yue Liu, Simon Krebs, Fuli Deng, Andreas Jentys, Debra J. Searles, M. Ali Haider, Rachit Khare, Johannes A. Lercher
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Structural Basis for Parallel G-Quadruplex Recognition by an Ankyrin Protein J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Khac Huy Ngo, Chong Wai Liew, Brahim Heddi, Anh Tuân Phan
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Chemical Potential Analysis as an Alternative to the van’t Hoff Method: Hypothetical Limits of Solar Thermochemical Hydrogen J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Stephan Lany
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Competing Reaction Mechanisms of Peptide Bond Formation in Water Revealed by Deep Potential Molecular Dynamics and Path Sampling J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Rolf David, Iñaki Tuñón, Damien Laage
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Triplet-Mediator Ligand-Protected Metal Nanocluster Sensitizers for Photon Upconversion J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-13 Daichi Arima, Shion Hidaka, So Yokomori, Yoshiki Niihori, Yuichi Negishi, Ryuichi Oyaizu, Takumi Yoshinami, Kenji Kobayashi, Masaaki Mitsui
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Combined Computational and Experimental Study Reveals Complex Mechanistic Landscape of Brønsted Acid-Catalyzed Silane-Dependent P═O Reduction J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-12 Jingyang Zhang, Wang-Yeuk Kong, Wentao Guo, Dean J. Tantillo, Yefeng Tang
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Extraordinary Electrical Conductance through Amorphous Nonconducting Polymers under Vibrational Strong Coupling J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-12 Sunil Kumar, Subha Biswas, Umar Rashid, Kavya S. Mony, Gokul Chandrasekharan, Francesco Mattiotti, Robrecht M. A. Vergauwe, David Hagenmuller, Veerabhadrarao Kaliginedi, Anoop Thomas
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Unlocking Direct Lithium Extraction in Harsh Conditions through Thiol-Functionalized Metal–Organic Framework Subnanofluidic Membranes J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-11 Chen Zhao, Fan Feng, Jue Hou, Jian Hu, Yuyu Su, Jefferson Zhe Liu, Matthew Hill, Benny D. Freeman, Huanting Wang, Huacheng Zhang
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An Uncommon Phosphorylation Mode Regulates the Activity and Protein Interactions of N-Acetylglucosamine Kinase J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-11 Arif Celik, Ida Beyer, Dorothea Fiedler
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Single Molecular Nanomedicines Based on Macrocyclic Carrier-Drug Conjugates for Concentration-Independent Encapsulation and Precise Activation of Drugs J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-11 Shun-Yu Yao, An-Kang Ying, Ze-Tao Jiang, Yuan-Qiu Cheng, Wen-Chao Geng, Xin-Yue Hu, Kang Cai, Dong-Sheng Guo
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Efficient Green Spin Light-Emitting Diodes Enabled by Ultrafast Energy- and Spin-Funneling in Chiral Perovskites J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Jingwen Yao, Zhiyu Wang, Yuling Huang, Jie Xue, Dengliang Zhang, Jiangshan Chen, Xihan Chen, Shou-Cheng Dong, Haipeng Lu
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A Robust Pyrazolate Metal–Organic Framework for Efficient Catalysis of Dehydrogenative C–O Cross Coupling Reaction J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-09 Rong-Ran Liang, Zongsu Han, Peiyu Cai, Yihao Yang, Joshua Rushlow, Zhaoyi Liu, Kun-Yu Wang, Hong-Cai Zhou
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Skeletal Formation of Carbocycles with CO2: Selective Synthesis of Indolo[3,2-b]carbazoles or Cyclophanes from Indoles, CO2, and Phenylsilane J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-09 Sha Li, Shoko Nakahara, Taishin Adachi, Takumi Murata, Kazuto Takaishi, Tadashi Ema
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Characterization of Deformational Isomerization Potential and Interconversion Dynamics with Ultrafast X-ray Solution Scattering J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Natalia E. Powers-Riggs, Benedikt O. Birgisson, Sumana L. Raj, Elisa Biasin, Philipp Lenzen, Diana Bregenholt Zederkof, Morten Haubro, Dagrún K. V. Tveiten, Robert W. Hartsock, Tim B. van Driel, Kristjan Kunnus, Matthieu Chollet, Joseph S. Robinson, Silke Nelson, Ruaridh Forbes, Kristoffer Haldrup, Kasper S. Pedersen, Gianluca Levi, Asmus Ougaard Dohn, Hannes Jónsson, Klaus Braagaard Mo̷ller, Adi Natan
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Photoresponsive Biomimetic Functions by Light-Driven Molecular Motors in Three Dimensionally Printed Liquid Crystal Elastomers J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Guiying Long, Yanping Deng, Wei Zhao, Guofu Zhou, Dirk J. Broer, Ben L. Feringa, Jiawen Chen
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Circular Heterochiral Titanium-Based Self-Assembled Architectures J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Pierre Mobian, David-Jérôme Pham, Alain Chaumont, Laurent Barloy, Georges Khalil, Nathalie Kyritsakas
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Resistive Memristors Using Robust Electropolymerized Porous Organic Polymer Films as Switchable Materials J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 You Tao, Hui Liu, Hui-Yuan Kong, Xin-Yue Bian, Bin-Wei Yao, Yong Jun Li, Cheng Gu, Xuesong Ding, Lianfeng Sun, Bao-Hang Han
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CO2-Based Stable Porous Metal–Organic Frameworks for CO2 Utilization J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Bo Song, Yuhang Liang, Yi Zhou, Liang Zhang, He Li, Neng-Xiu Zhu, Ben Zhong Tang, Dan Zhao, Bin Liu
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Multivariate Bayesian Optimization of CoO Nanoparticles for CO2 Hydrogenation Catalysis J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Lanja R. Karadaghi, Emily M. Williamson, Anh T. To, Allison P. Forsberg, Kyle D. Crans, Craig L. Perkins, Steven C. Hayden, Nicole J. LiBretto, Frederick G. Baddour, Daniel A. Ruddy, Noah Malmstadt, Susan E. Habas, Richard L. Brutchey
The hydrogenation of CO2 holds promise for transforming the production of renewable fuels and chemicals. However, the challenge lies in developing robust and selective catalysts for this process. Transition metal oxide catalysts, particularly cobalt oxide, have shown potential for CO2 hydrogenation, with performance heavily reliant on crystal phase and morphology. Achieving precise control over these
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Modular Access to Chiral Amines via Imine Reductase-Based Photoenzymatic Catalysis J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Bin Chen, Renjie Li, Jianqiang Feng, Beibei Zhao, Jiawei Zhang, Jinhai Yu, Yuanyuan Xu, Zhongqiu Xing, Yue Zhao, Binju Wang, Xiaoqiang Huang
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Darobactin Substrate Engineering and Computation Show Radical Stability Governs Ether versus C–C Bond Formation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Austin M. Woodard, Francesca Peccati, Claudio D. Navo, Gonzalo Jiménez-Osés, Douglas A. Mitchell
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A Method for Rigorously Selective Capture and Simultaneous Fluorescent Labeling of N-Terminal Glycine Peptides J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Hongxu Liu, Harnimarta Deol, Ava Raeisbahrami, Hadis Askari, Christopher D. Wight, Vincent M. Lynch, Eric V. Anslyn
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Carbene-Stabilized Phosphagermylenylidene: A Heavier Analog of Isonitrile J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Jiancheng Li, Xin-Feng Wang, Chaopeng Hu, Liu Leo Liu
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Stimulus-Induced Dynamic Behavior Regulation of Flexible Crystals through the Tuning of Module Rigidity J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-10 Han Fang, Xiao-Yi Liu, Hao-Jing Ding, Meagan Mulcair, Brian Space, Hongliang Huang, Xing-Wang Li, Shu-Ming Zhang, Mei-Hui Yu, Ze Chang, Xian-He Bu
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Superconductivity above 105 K in Nonclathrate Ternary Lanthanum Borohydride below Megabar Pressure J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-09 Xiaoxu Song, Xiaokuan Hao, Xudong Wei, Xin-Ling He, Hanyu Liu, Liang Ma, Guangtao Liu, Hongbo Wang, Jingyu Niu, Shaojie Wang, Yanpeng Qi, Zhongyuan Liu, Wentao Hu, Bo Xu, Lin Wang, Guoying Gao, Yongjun Tian
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Structural Insights into Seeding Mechanisms of hIAPP Fibril Formation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-09 Saba Suladze, Christian Sustay Martinez, Diana C. Rodriguez Camargo, Jonas Engler, Natalia Rodina, Riddhiman Sarkar, Martin Zacharias, Bernd Reif
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Biocompatible Tough Ionogels with Reversible Supramolecular Adhesion J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-05-09 Jiaofeng Xiong, Minzhi Duan, Xiuyang Zou, Shuna Gao, Jiangna Guo, Xiaowei Wang, Qingning Li, Weizheng Li, Xiaoliang Wang, Feng Yan